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Measurements of individual and ensemble lifetimes of high-lying Rb Rydberg states

Abstract

We demonstrate a hybrid method based on field ionization and state-selective de-excitation capable of measuring the lifetimes of high-lying Rydberg states. For nS Rydberg states of Rb atoms with principal quantum number 60≤ n≤88, we measure both the individual target state lifetimes and those of the ensemble of Rydberg states populated via black-body radiation-induced transitions. We find good overall agreement with numerical calculations of the expected lifetimes in both cases. However, for the target state lifetimes, we find a local deviation towards shorter lifetimes for states around n=72, which we interpret as a signature of a modified black-body spectrum in the finite volume in which our experiments take place.

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