Abstract
Periodic driving can tune the quasistatic properties of quantum matter. A well-known example is the dynamical modification of tunneling by an oscillating electric field. Here we show experimentally that driving the phasonic degree of freedom of a cold-atom quasicrystal can continuously tune the effective quasi-disorder strength, reversibly toggling a localization-delocalization quantum phase transition. Measurements agree with fit-parameter-free theoretical predictions, and illuminate a fundamental connection between Aubry-Andr\'e localization in one dimension and dynamic localization in the associated two-dimensional Harper-Hofstadter model. These results open up new experimental possibilities for dynamical coherent control of quantum phase transitions.