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Enhancement of optical coherence in ¹67Er:Y₂SiO₅ crystal at sub-Kelvin temperatures

Abstract

Er³⁺:Y₂SiO₅ crystal is a promising candidate with a great variety of its potential applications in quantum information processing and quantum communications ranging from optical/microwave quantum memories to circuit QED and microwave-to-optics frequency converters. Some of the above listed applications require ultra-low temperature environment, i.e., temperatures T0.1 K. Most of the experiments with erbium doped crystals have been so far carried out at temperatures above 1.5~K. Therefore, only little information is known about Er³⁺:Y₂SiO₅ coherence properties at millikelvins. Here, we investigate optical decoherence of ¹⁶⁷Er:Y₂SiO₅ crystal by performing 2- and 3-pulse echo experiments at millikelvin temperature range and at weak and moderate magnetic fields. We show that the deep freezing of the crystal results in an increase of optical coherence time by one order of magnitude compared to temperature of 1.5 Kelvin and magnetic field of ∼0.2~T, taken as a reference point. We further describe the detailed investigation of the decoherence mechanisms in this regime.

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